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Polydimethylsiloxane assisted supercritical CO

Weixia Wang, Shuai Zhou, Zhong Xin, Yaoqi Shi, Shicheng Zhao

Frontiers of Chemical Science and Engineering 2016, Volume 10, Issue 3, Pages 396-404 doi: 10.1007/s11705-016-1577-z

Abstract: The effect of PDMS viscosity on the foaming behavior of HMSPP was systematically investigated using supercritical

Keywords： high melt strength polypropylene (HMSPP) polydimethylsiloxane (PDMS) supercritical CO2sub> foaming

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Chemical reactions of oily sludge catalyzed by iron oxide under supercritical water gasification condition

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 6, Pages 886-896 doi: 10.1007/s11705-021-2125-z

Abstract: To evaluate the mechanism of Fe2sub>O3sub> catalyst and the migration pathways of heteroatomsIn terms of the catalytic mechanisms of Fe2sub>O3sub>, the surface lattice oxygen is consumedby small carbon fragments to produce CO and CO2sub>, improving the catalytic performance of theThe heteroatom O was removed under the effects of supercritical water.Heavy metal particles presented in the oily sludge, such as iron in association with Fe2sub>O<

Keywords： oily sludge SCWG ReaxFF Fe2sub>O3sub> heteroatoms

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Thermo-economic analysis of a direct supercritical CO electric power generation system using geothermal

Frontiers in Energy 2022, Volume 16, Issue 2, Pages 246-262 doi: 10.1007/s11708-021-0749-9

Abstract: A comprehensive thermo-economic model combining a geothermal heat mining system and a direct supercriticalCO2sub> turbine expansion electric power generation system was proposed in this paper.>2sub> injection flowrate, CO2sub> injection temperature, and monitored production well bottoma 20-year steady operation without considering CO2sub> sequestration credit.In addition, when CO2sub> sequestration credit is $1.00/t, an LCOE breakeven point compared to

Keywords： geothermal heat mining supercritical CO2sub> power generation thermo-economic analysis optimization

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Key problems and solutions in supercritical CO

Haizhu WANG, Gensheng LI, Bin ZHU, Kamy SEPEHRNOORI, Lujie SHI, Yong ZHENG, Xiaomei SHI

Frontiers in Energy 2019, Volume 13, Issue 4, Pages 667-672 doi: 10.1007/s11708-019-0626-y

Abstract: Supercritical CO fracturing is considered to be a new method for efficient exploitation of unconventionalSupercritical CO has many special properties including low viscosity, high diffusion coefficient, andthe problem of poor capacity in proppant carrying and sand plug, the methods of adding tackifier into supercriticalAfter solving the above three problems, the field test of supercritical CO fracturing can be conductedThe research results can promote the industrialization process of supercritical CO fracturing.

Keywords： supercritical CO2sub> fracturing friction loss proppant carrying flied test problem

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Preliminary experimental study of a supercritical CO

Junhyun CHO, Hyungki SHIN, Jongjae CHO, Young-Seok KANG, Ho-Sang RA, Chulwoo ROH, Beomjoon LEE, Gilbong LEE, Byunghui KIM, Young-Jin BAIK

Frontiers in Energy 2017, Volume 11, Issue 4, Pages 452-460 doi: 10.1007/s11708-017-0504-4

Abstract: Research on applying a supercritical carbon dioxide power cycle (S-CO ) to concentrating solar powerA basic sub-kWe class test loop with a high-speed radial type turbo-generator and a test loop with aBy operating the sub-kWe class test loop using R134a as the working fluid instead of CO , an average

Keywords： supercritical CO2sub> power cycle turbomachinery compressor turbine

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Calculation and analysis of sub/supercritical methanol preheating tube for continuous production of biodieselvia supercritical methanol transesterification

Wen CHEN, Weiyong YING, Cunwen WANG, Weiguo WANG, Yuanxin WU, Junfeng ZHANG,

Frontiers in Energy 2009, Volume 3, Issue 4, Pages 423-431 doi: 10.1007/s11708-009-0075-0

Abstract: Supercritical methanol transesterification for biodiesel has recently been concerned because of its obvious#8213;600K, changes of the density, isobaric capacity, viscosity and thermal conductivity of sub/supercritical methanol with temperature are first discussed.on the basis of these thermophysical properties, an integration method is adopted for the design of subcomputational results show that the Reynolds number and the local convection heat-transfer coefficient of sub

Keywords： sub/supercritical methanol preheating tube integration method biodiesel

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Preliminary design of an SCO conversion system applied to the sodium cooled fast reactor

Frontiers in Energy 2021, Volume 15, Issue 4, Pages 832-841 doi: 10.1007/s11708-021-0777-5

Abstract: The supercritical carbon dioxide (SCO2sub>) Brayton cycle has become an ideal power conversionIn this paper, the 1200 MWesub> large pool SFR (CFR1200) is used as the heat source of the systemThe performance of different SCO2sub> Brayton cycle systems and changes in key equipment performancenuclear island adopts the flow-advanced operation strategy and the carbon dioxide flowrate in the SCO2sub> power conversion system is adjusted with the goal of maintaining the sodium-carbon dioxide heat

Keywords： sodium-cooled fast reactor (SFR) supercritical carbon dioxide (SCO2sub>) brayton cycle load

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Biodiesel production from waste frying oil in sub- and supercritical methanol on a zeolite Y solid acid

Jorge MEDINA-VALTIERRA, Jorge RAMIREZ-ORTIZ

Frontiers of Chemical Science and Engineering 2013, Volume 7, Issue 4, Pages 401-407 doi: 10.1007/s11705-013-1354-1

Abstract: In this study biodiesel was produced from WFO in sub- and super-critical methanol on a zeolite Y solid

Keywords： biodiesel methanol critical temperature waste frying oil zeolite Y

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Rh2sub>O3sub>/hexagonal CePO4sub> nanocatalysts for N2sub>O decomposition

Huan Liu, Zhen Ma

Frontiers of Chemical Science and Engineering 2017, Volume 11, Issue 4, Pages 586-593 doi: 10.1007/s11705-017-1659-6

Abstract: Hexagonal CePO nanorods were prepared by a precipitation method and hexagonal CePO nanowires were prepared by hydrothermal synthesis at 150 °C. Rh(NO ) was then used as a precursor for the impregnation of Rh O onto these CePO materials. The Rh O supported on the CePO nanowires was much more active for the catalytic decomposition of N O than the Rh O supported on CePO nanorods. The stability of both catalysts as a function of time on stream was studied and the influence of the co-feed (CO , O , H O or O /H O) on the N O decomposition was also investigated. The samples were characterized by N adsorption-desorption, inductively coupled plasma optical emission spectroscopy, X-ray diffraction, transmission electron microscopy, X-ray photoelectron microscopy, hydrogen temperature-programmed reduction, oxygen temperature-programmed desorption, and CO temperature-programmed desorption in order to correlate the physicochemical and catalytic properties.

Keywords： Rh2sub>O3sub> CePO4sub> N2sub>O decomposition

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CO2sub> methanation and co-methanation of CO and CO2sub> over Mn-promoted Ni/Al2sub>O3sub> catalysts

Kechao Zhao,Zhenhua Li,Li Bian

Frontiers of Chemical Science and Engineering 2016, Volume 10, Issue 2, Pages 273-280 doi: 10.1007/s11705-016-1563-5

Abstract: A series of Mn-promoted 15 wt-% Ni/Al O catalysts were prepared by an incipient wetness impregnation method. The effect of the Mn content on the activity of the Ni/Al O catalysts for CO methanation and the co-methanation of CO and CO in a fixed-bed reactor was investigated. The catalysts were characterized by N physisorption, hydrogen temperature-programmed reduction and desorption, carbon dioxide temperature-programmed desorption, X-ray diffraction and high-resolution transmission electron microscopy. The presence of Mn increased the number of CO adsorption sites and inhibited Ni particle agglomeration due to improved Ni dispersion and weakened interactions between the nickel species and the support. The Mn-promoted 15 wt-% Ni/Al O catalysts had improved CO methanation activity especially at low temperatures (250 to 400 °C). The Mn content was varied from 0.86% to 2.54% and the best CO conversion was achieved with the 1.71Mn-Ni/Al O catalyst. The co-methanation tests on the 1.71Mn-Ni/Al O catalyst indicated that adding Mn markedly enhanced the CO methanation activity especially at low temperatures but it had little influence on the CO methanation performance. CO methanation was more sensitive to the reaction temperature and the space velocity than the CO methanation in the co-methanation process.

Keywords： Mn promotion nickel catalysts CO2sub> methanation co-methanation of CO and CO2sub>

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A Storage-Driven CO2sub> EOR for a Net-Zero Emission Target Article

Yueliang Liu, Zhenhua Rui

Engineering 2022, Volume 18, Issue 11, Pages 79-87 doi: 10.1016/j.eng.2022.02.010

Abstract: >2sub>) emissions.>2sub> emissions by storing CO2sub> in oil reservoirs.CO2sub> EOR—whose main target is to realize net-zero or even negative CO2sub> emissionsStorage-driven CO2sub> EOR is superior to conventional CO2sub> EOR in improving sweepingthan conventional CO2sub> EOR.

Keywords： CO2sub> EOR Net CO2sub> emissions Dimethyl ether Storage-driven CO2sub> EOR CO2sub> sequestration

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Al2sub>O3sub> and CeO2sub>-promoted MgO sorbents for CO2sub> capture at moderate

Huimei Yu, Xiaoxing Wang, Zhu Shu, Mamoru Fujii, Chunshan Song

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 1, Pages 83-93 doi: 10.1007/s11705-017-1691-6

Abstract: A series of Al O and CeO modified MgO sorbents was prepared and studied for CO sorption at moderate temperatures. The CO sorption capacity of MgO was enhanced with the addition of either Al O or CeO . Over Al O -MgO sorbents, the best capacity of 24.6 mg-CO /g-sorbent was attained at 100 °C, which was 61% higher than that of MgO (15.3 mg-CO /g-sorbent). The highest capacity of 35.3 mg-CO /g-sorbent was obtained over the CeO -MgO sorbents at the optimal temperature of 200 °C. Combining with the characterization results, we conclude that the promotion effect on CO sorption with the addition of Al O and CeO can be attributed to the increased surface area with reduced MgO crystallite size. Moreover, the addition of CeO increased the basicity of MgO phase, resulting in more increase in the CO capacity than Al O promoter. Both the Al O -MgO and CeO -MgO sorbents exhibited better cyclic stability than MgO over the course of fifteen CO sorption-desorption cycles. Compared to Al O , CeO is more effective for promoting the CO capacity of MgO. To enhance the CO capacity of MgO sorbent, increasing the basicity is more effective than the increase in the surface area.

Keywords： CO2sub> capture MgO sorbents Al2sub>O3sub> CeO2sub> flue gas

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The stabilization effect of Al2sub>O3sub> on unconventional Pb/SiO2sub> catalyst

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10, Pages 1423-1429 doi: 10.1007/s11705-023-2315-y

Abstract: To enhance the stability, the traditional carrier Al2sub>O3sub> with a small amount, wasintroduced into Pb/SiO2sub> catalyst in this study.It has been proved that Al2sub>O3sub> can inhibit the reduction of PbO, and weaken theAs a result, 3Al15Pb/SiO2sub> catalyst exhibits a much higher stability up to more than 150 h.>2sub>O3sub> addition was also proposed.

Keywords： Pb/SiO2sub> Al2sub>O3sub> propane dehydrogenation propene stability

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Cu-doped Bi/Bi2sub>WO6sub> catalysts for efficient N2sub> fixation by photocatalysis

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10, Pages 1412-1422 doi: 10.1007/s11705-023-2312-1

Abstract: it in photocatalytic N2sub> immobilization.>2sub>WO6sub> composite.>2sub>WO6sub>.>2sub>WO6sub>, respectively.>2sub>-to-NH3sub> conversion.

Keywords： Bi2sub>WO6sub> Cu doping work function photocatalytic N2sub> fixation charge

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ZnFe2sub>O4sub> deposited on BiOCl with exposed (001) and (010) facets for photocatalyticreduction of CO2sub> in cyclohexanol

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

Frontiers of Chemical Science and Engineering 2017, Volume 11, Issue 2, Pages 197-204 doi: 10.1007/s11705-016-1606-y

Abstract: ZnFe O -BiOCl composites were prepared by both hydrothermal and direct precipitation processes and the structures and properties of the samples were characterized by various instrumental techniques. The samples were then used as catalysts for the photocatalytic reduction of CO in cyclohexanol under ultraviolet irradiation to give cyclohexanone (CH) and cyclohexyl formate (CF). The photocatalytic CO reduction activities over the hydrothermally prepared ZnFe O -BiOCl composites were higher than those over the directly-precipitated composites. This is because compared to the direct-precipitation sample, the ZnFe O nanoparticles in the hydrothermal sample were smaller and more uniformly distributed on the surface of BiOCl and so more heterojunctions were formed. Higher CF and CH yields were obtained for the pure BiOCl and BiOCl composite samples with more exposed (001) facets than for the samples with more exposed (010) facets. This is due to the higher density of oxygen atoms in the exposed (001) facets, which creates more oxygen vacancies, and thereby improves the separation efficiency of the electron-hole pairs. More importantly, irradiation of the (001) facets with ultraviolet light produces photo-generated electrons which is helpful for the reduction of CO to ·CO . The mechanism for the photocatalytic reduction of CO in cyclohexanol over ZnFe O -BiOCl composites with exposed (001) facets involves electron transfer and carbon radical formation.

Keywords： reduction of CO2sub> cyclohexanol ZnFe2sub>O4sub> deposited BiOCl facet composite

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Title Author Date Type Operation

Polydimethylsiloxane assisted supercritical CO

Weixia Wang, Shuai Zhou, Zhong Xin, Yaoqi Shi, Shicheng Zhao

Journal Article

Chemical reactions of oily sludge catalyzed by iron oxide under supercritical water gasification condition

Journal Article

Thermo-economic analysis of a direct supercritical CO electric power generation system using geothermal

Journal Article

Key problems and solutions in supercritical CO

Haizhu WANG, Gensheng LI, Bin ZHU, Kamy SEPEHRNOORI, Lujie SHI, Yong ZHENG, Xiaomei SHI

Journal Article

Preliminary experimental study of a supercritical CO

Junhyun CHO, Hyungki SHIN, Jongjae CHO, Young-Seok KANG, Ho-Sang RA, Chulwoo ROH, Beomjoon LEE, Gilbong LEE, Byunghui KIM, Young-Jin BAIK

Journal Article

Calculation and analysis of sub/supercritical methanol preheating tube for continuous production of biodieselvia supercritical methanol transesterification

Wen CHEN, Weiyong YING, Cunwen WANG, Weiguo WANG, Yuanxin WU, Junfeng ZHANG,

Journal Article

Preliminary design of an SCO conversion system applied to the sodium cooled fast reactor

Journal Article

Biodiesel production from waste frying oil in sub- and supercritical methanol on a zeolite Y solid acid

Jorge MEDINA-VALTIERRA, Jorge RAMIREZ-ORTIZ

Journal Article

Rh2sub>O3sub>/hexagonal CePO4sub> nanocatalysts for N2sub>O decomposition

Huan Liu, Zhen Ma

Journal Article

CO2sub> methanation and co-methanation of CO and CO2sub> over Mn-promoted Ni/Al2sub>O3sub> catalysts

Kechao Zhao,Zhenhua Li,Li Bian

Journal Article

A Storage-Driven CO2sub> EOR for a Net-Zero Emission Target

Yueliang Liu, Zhenhua Rui

Journal Article

Al2sub>O3sub> and CeO2sub>-promoted MgO sorbents for CO2sub> capture at moderate

Huimei Yu, Xiaoxing Wang, Zhu Shu, Mamoru Fujii, Chunshan Song

Journal Article

The stabilization effect of Al2sub>O3sub> on unconventional Pb/SiO2sub> catalyst

Journal Article

Cu-doped Bi/Bi2sub>WO6sub> catalysts for efficient N2sub> fixation by photocatalysis

Journal Article

ZnFe2sub>O4sub> deposited on BiOCl with exposed (001) and (010) facets for photocatalyticreduction of CO2sub> in cyclohexanol

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

Journal Article

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